Anime isn't as cool as film, but if you're looking for some decent anime...
Series:
- Samurai Champloo
- Big-O
- Outlaw Star
- Deathnote
- Wolf's Rain
- FLCL
- Samurai 7
- Fullmetal Alchemist
Films:
- Princess Mononoke
- Spirited Away
- Howl's Moving Castle
- Fullmetal Alchemist
- Ninja Scroll